| 1 | Big Ben (London Films) | [no artist] | 0:18 |
| 2 | The Harry Lime Theme | Gertrud Huber | 2:21 |
| 3 | "It's a Shame" (dialogue) | Trevor Howard & Joseph Cotten | 0:14 |
| 4 | The Café Mozart Waltz | Gertrud Huber | 2:24 |
| 5 | Main Title - Harry's False Funeral | Gertrud Huber | 5:58 |
| 6 | "Heard of Harry Lime?" (dialogue) | Joseph Cotten & Wilfrid Hyde‐White | 0:09 |
| 7 | Holly Encounters Anna / Meeting the Conspirators | Gertrud Huber | 3:01 |
| 8 | "The Third Man" (dialogue) | Trevor Howard & Joseph Cotten | 0:35 |
| 9 | Holly Is Accused of Homicide | Gertrud Huber | 2:31 |
| 10 | "This Isn't Santa Fe" (dialogue) | Trevor Howard & Joseph Cotten | 0:20 |
| 11 | Holly Brings Flowers | Gertrud Huber | 6:15 |
| 12 | Holly Runs After Harry's Shadow | Gertrud Huber | 4:56 |
| 13 | "Holly, What Fools We Are" (dialogue) | Orson Welles & Joseph Cotten | 0:45 |
| 14 | Trap to Catch Harry | Gertrud Huber | 3:33 |
| 15 | "The Cuckoo Clock" (dialogue) | Orson Welles | 0:23 |
| 16 | Anna Walks Away / End Title: The Harry Lime Theme | Gertrud Huber | 4:10 |
| 17 | Visions of Vienna | Gertrud Huber | 1:59 |
| 18 | Danube Dreams | Gertrud Huber | 2:19 |
| 19 | The Harry Lime Theme (bonus: orchestral version) | The City of Prague Philharmonic Orchestra, Nic Raine | 2:35 |
| 20 | The Café Mozart Waltz (bonus: orchestral version) | The City of Prague Philharmonic Orchestra, Nic Raine | 3:15 |