| 1 | Nature Boy (original mono LP mix) | Marvin Gaye | 2:52 |
| 2 | Ramblin Rose (original mono LP mix) | Marvin Gaye | 2:51 |
| 3 | Too Young (original mono LP mix) | Marvin Gaye | 3:48 |
| 4 | Pretend (original mono LP mix) | Marvin Gaye | 2:50 |
| 5 | Straighten Up and Fly Right (original mono LP mix) | Marvin Gaye | 2:25 |
| 6 | Mona Lisa (original mono LP mix) | Marvin Gaye | 3:04 |
| 7 | Unforgettable (original mono LP mix) | Marvin Gaye | 3:43 |
| 8 | To the Ends of the Earth (original mono LP mix) | Marvin Gaye | 2:23 |
| 9 | Sweet Lorraine (original mono LP mix) | Marvin Gaye | 2:50 |
| 10 | It’s Only a Paper Moon (original mono LP mix) | Marvin Gaye | 2:29 |
| 11 | Send for Me (original mono LP mix) | Marvin Gaye | 2:37 |
| 12 | Calypso Blues (original mono LP mix) | Marvin Gaye | 4:08 |
| 13 | Unforgettable (original California version, take 2) | Marvin Gaye | 4:03 |
| 14 | Send for Me (original Cali version, take 1) | Marvin Gaye | 2:56 |
| 15 | Send for Me (original Cali version, take 3) | Marvin Gaye | 2:46 |
| 16 | Ramblin’ Rose (alternate vocal) | Marvin Gaye | 2:52 |
| 17 | Too Young (alternate vocal, take 1) | Marvin Gaye | 3:49 |
| 18 | Send for Me (alternate vocal, take 1) | Marvin Gaye | 3:17 |
| 19 | The More I See You | Marvin Gaye | 2:33 |
| 20 | I Wish You Love | Marvin Gaye | 3:38 |
| 21 | The End of a Love Affair | Marvin Gaye | 3:22 |
| 22 | Violets for Your Furs | Marvin Gaye | 4:14 |
| 23 | So in Love | Marvin Gaye | 2:38 |
| 24 | If I Had to Go | Marvin Gaye | 3:12 |
| 25 | You’re All That Matter to Me | Marvin Gaye | 2:35 |
| 26 | Goodbye | Marvin Gaye | 2:48 |