| 1 | Puff, the Magic Dragon | Peter, Paul and Mary | 3:25 |
| 2 | My Brother | Terry Scott | 2:37 |
| 3 | There's A Hole In My Bucket | Harry Belafonte | 4:20 |
| 4 | Right Said Fred | Bernard Cribbins | 2:19 |
| 5 | Nellie The Elephant | Mandy Miller | 2:31 |
| 6 | English Country Garden | Jimmie Rodgers | — |
| 7 | Don't Jump off the Roof Dad | Tommy Cooper | — |
| 8 | I've Got No Strings (From Pinnochio) | Dickie Jones | 2:24 |
| 9 | Hippopotamus Song (Mud Mud Glorious Mud) | Michael Flanders and Donald Swann | 2:54 |
| 10 | When You Wish Upon A Star (from Pinnochio) | Cliff Edwards | 3:16 |
| 11 | My Boomerang Won't Come Back | Charlie Drake | — |
| 12 | Who's Afraid Of The Big Bad Wolf | Pinky & Perky | — |
| 13 | The Laughing Policeman | Charles Penrose | 2:38 |
| 14 | The Siamese Cat Song (from Lady And The Tramp) | Peggy Lee | 2:13 |
| 15 | The Ugly Duckling | Danny Kaye | — |
| 16 | Give A Litlte Whistle (from Pinnochio) | Cliff Edwards & Dickie Jones | — |
| 17 | Tie Me Kangaroo Down Sport | Rolf Harris | 2:44 |
| 18 | What a Mouth (What a North and South) | Tommy Steele | — |
| 19 | The Ugly Bug Ball | Burl Ives | 2:59 |
| 20 | Zip A Dee Doo Dah (From Song Of The South) | James Baskett | 2:17 |
| 21 | When I See An Elephant Fly (from Dumbo) | Cliff Edwards & The Hall Johnson Singers | — |
| 22 | I Taut I Taw a Puddy Tat | Mel Blanc | 2:59 |
| 23 | Tubby the Tuba | Danny Kaye | — |
| 24 | The Gnu | Michael Flanders and Donald Swann | 2:46 |
| 25 | The Runaway Train | Michael Holliday | 2:11 |
| 26 | You're a Pink Toothbrush | Max Bygraves | 2:30 |
| 27 | The Hole in the Ground | Bernard Cribbins | 1:52 |
| 28 | Puffin' Billy | Melodi Light Orchestra | 2:57 |
| 29 | The Teccy Bears Picnic | Pinky & Perky | 2:18 |
| 30 | The Mole in the Hole | The Southlanders | — |
| 31 | High Hopes | Frank Sinatra | 2:43 |
| 32 | Meet the Flintstones | Hoyt Curtin | 0:41 |
| 33 | Busy Doing Nothing- from 'A Connecticut Yankee In King Arthur's Court' | Bing Crosby | 2:56 |
| 34 | The Lion and Albert | Stanley Holloway | 3:14 |
| 35 | Food Glorious Food | Keith Hampshire & Cast Of Oliver | — |
| 36 | The Inchworm | Danny Kaye | 3:11 |
| 37 | The Little White Bull | Tommy Steele | 3:45 |
| 38 | Once Upon a Dream (From Cinderella) | Bill Shirley & Mary Costa | — |
| 39 | Pop Goes the Weasel | Anthony Newley | 2:46 |
| 40 | Top Cat (Main Title) | Hoyt Curtin | 0:45 |
| 41 | Car Song | Woody Guthrie | 1:51 |
| 42 | Thumbelina | Danny Kaye | — |
| 43 | Ali Baba's Camel | The Rhythmic Troubadours | 3:02 |
| 44 | When You Come to the End of a Lollipop | Max Bygraves | 2:40 |
| 45 | I've Been Everywhere (Walkers Crisps TV Ad) | The Mudlarks | — |
| 46 | The Dance Of The Cuckoos- Laurel and Hardy Theme | Laurel & Hardy | 0:28 |
| 47 | Morningtown Ride | The Limeliters | 2:54 |
| 48 | Animal Magic (Las Vegas) Original Theme | Laurie Johnson | 2:23 |
| 49 | Twenty Tiny Fingers | Alma Cogan | 2:36 |
| 50 | Do Re Mi- from 'The Sound Of Music' | Mary Martin | 5:51 |
| 51 | Speedy Gonzales | Pat Boone | 2:39 |
| 52 | Charlie Brown | The Coasters | 2:19 |
| 53 | Me And My Shadow | Morecambe & Wise | 2:33 |
| 54 | I'm Glad That I'm Bugs Bunny | Mel Blanc | — |
| 55 | Hello My Darlings | Charlie Drake | — |
| 56 | Woody Woodpecker (Main Theme) | The Warner Brothers Orchestra | 0:48 |
| 57 | Tom and Jerry (Main Theme) | The Warner Brothers Orchestra | 0:25 |
| 58 | Strawberry Fair | Anthony Newley | 2:18 |
| 59 | I Can't Do My Bally Bottom Button Up | Ian Wallace | 2:49 |
| 60 | Sugartime | Alma Cogan | 1:49 |
| 61 | Oranges And Lemons | Uncle Mac | — |
| 62 | Christopher Robin At Buckingham Palace | Petula Clark | 2:11 |
| 63 | How Much Is That Doggie in the Window | Lita Roza | — |
| 64 | Robin Hood | Dick James | 2:31 |
| 65 | Gilly Gilly Ossenfeffer Katzenellenbogen by the Sea | Max Bygraves | — |
| 66 | Little Boy Fishing | Shirley Abicair | 2:45 |
| 67 | The Deadwood Stage | Doris Day | — |
| 68 | Dance Duet (Hansel And Gretel) | Manchester Children's Choir | 3:11 |
| 69 | Bluebell Polka | Jimmy Shand | 2:24 |
| 70 | Donald Where's Your Troosers? | Andy Stewart | — |
| 71 | The Typewriter | Leroy Anderson | 1:40 |
| 72 | Christopher Robin Is Saying His Prayers | Ann Stephens | 2:17 |
| 73 | Heigh Ho (from Snow White and the Seven Dwarves) | The Dwarf Chorus | — |
| 74 | Seven Little Girls Sitting in the Back Seat | The Avons | 2:14 |
| 75 | Standing on the Corner | The King Brothers | 2:44 |
| 76 | Where Will The Dimple Be | Alma Cogan | 2:19 |
| 77 | I Know an Old Lady | Burl Ives | 2:41 |
| 78 | Any Old Iron | Peter Sellers | 2:54 |
| 79 | The King's New Clothes | Danny Kaye | — |
| 80 | Grasshopper Dance | Jack Hylton | 3:20 |
| 81 | Michael Row The Boat Ashore | The Highwaymen | — |
| 82 | Where Have All The Flowers Gone | The Kingston Trio | 3:04 |
| 83 | Zambesi | Lou Busch | 2:38 |
| 84 | Carbon the Copycat | Tex Ritter | 2:44 |
| 85 | Sparky's Magic Echo | Henry Blair | 6:19 |
| 86 | Sixteen Tons | Tennessee Ernie Ford | 2:36 |
| 87 | Big Rock Candy Mountain | Burl Ives | 1:41 |
| 88 | Soldier Won't You Marry Me | Jimmie Rodgers | — |
| 89 | Little Sir Echo | Max Bygraves | 2:08 |
| 90 | The Little Shoemaker | The Michael Twins | 2:28 |
| 91 | Coronation Scot (Paul Temple Theme) | Sidney Torch | 3:00 |
| 92 | In the Middle of the House | Alma Cogan | 2:08 |
| 93 | The Happy Wanderer | The Obernkirchen Children's Choir | — |
| 94 | The Owl And The Pussycat | Elton Hayes | 2:19 |
| 95 | Little Red Monkey | Joy Nichols, Dick Bentley & Jimmy Edwards | 2:32 |
| 96 | Beep Beep | The Playmates | 3:04 |
| 97 | Kitty In The Basket | Diana Decker | 2:34 |
| 98 | Tom Dooley | The Kingston Trio | 2:29 |
| 99 | Ragtime Cowboy Joe | The Chipmunks | 2:06 |
| 100 | Pickin' a Chicken | Eve Boswell | — |