| 1 | L-O-V-E | Nat King Cole | 2:34 |
| 2 | Walkin' | Nat King Cole | 2:50 |
| 3 | (I Would Do) Anything for You | Nat King Cole | 1:46 |
| 4 | The Song is Ended (but the Melody Lingers On) | Nat King Cole | 2:46 |
| 5 | Unforgettable (1961 version) | Nat King Cole | 3:28 |
| 6 | Walkin' My Baby Back Home | Nat King Cole | 2:40 |
| 7 | I'm Gonna Sit Right Down (and Write Myself a Letter) | Nat King Cole | 2:37 |
| 8 | Midnight Flyer | Nat King Cole | 2:12 |
| 9 | Send for Me | Nat King Cole | 2:38 |
| 10 | Open Up the Doghouse (Two Cats Are Coming In) | Nat King Cole with Dean Martin | 2:27 |
| 11 | (Get Your Kicks on) Route 66 (1961 version) | Nat King Cole | 2:55 |
| 12 | Love | Nat King Cole | 2:02 |
| 13 | Papa Loves Mambo | Nat King Cole | 2:40 |
| 14 | You've Got the Indian Sign on Me | Nat King Cole | 1:48 |
| 15 | Mona Lisa | Nat King Cole | 3:27 |
| 16 | Let's Face the Music and Dance | Nat King Cole | 2:26 |
| 17 | Almost Like Being in Love | Nat King Cole | 1:54 |
| 18 | Don't Get Around Much Anymore | Nat King Cole | 3:11 |
| 19 | Orange Colored Sky | Nat King Cole | 2:33 |
| 20 | Long, Long Ago | Nat King Cole with Dean Martin | 2:18 |
| 21 | Breezin' Along With the Breeze | Nat King Cole | 2:30 |
| 22 | You're Wrong All Wrong | Nat King Cole | 2:57 |
| 23 | You Weren't There | Nat King Cole | 3:05 |
| 24 | How (How Do I Go About It?) | Nat King Cole | 2:45 |
| 25 | Sweet William (and Lily at the Valley) | Nat King Cole | 3:21 |
| 26 | Sleeping Beauty | Nat King Cole | 3:01 |
| 27 | When I'm Alone | Nat King Cole | 2:49 |
| 28 | The Magic Window | Nat King Cole | 3:23 |
| 29 | Little Fingers | Nat King Cole | 2:50 |
| 30 | Ain't She Sweet | Nat King Cole with Carole & Natalie Cole | 2:46 |
| 31 | What to Do | Nat King Cole with Carole & Natalie Cole | 2:33 |
| 32 | Straighten Up and Fly Right (alternate take) | Nat King Cole | 2:56 |
| 33 | (I Love You) For Sentimental Reasons (alternate take) | Nat King Cole | 3:25 |
| 34 | Unforgettable (alternate take) | Nat King Cole | 4:16 |
| 35 | Mona Lisa (alternate take) | Nat King Cole | 3:41 |
| 36 | The Christmas Song (alternate take) | Nat King Cole | 3:16 |