| 1 | Smile | Nat King Cole | 2:56 |
| 2 | It's Only a Paper Moon | The Nat King Cole Trio | 2:56 |
| 3 | Straighten Up and Fly Right | The Nat King Cole Trio | 2:27 |
| 4 | (Get Your Kicks on) Route 66 | The Nat King Cole Trio | 3:02 |
| 5 | You Stepped Out of a Dream | Nat King Cole | 2:36 |
| 6 | (I Love You) For Sentimental Reasons | The Nat King Cole Trio | 2:54 |
| 7 | Nature Boy | The Nat King Cole Trio | 2:40 |
| 8 | Too Young | Nat King Cole | 3:13 |
| 9 | Unforgettable | Nat King Cole | 3:12 |
| 10 | Walkin' My Baby Back Home | Nat King Cole | 2:41 |
| 11 | Orange Colored Sky | The Nat King Cole Trio / Stan Kenton and His Orchestra | 2:34 |
| 12 | Send for Me | Nat King Cole | 2:31 |
| 13 | Looking Back | Nat King Cole | 2:27 |
| 14 | A Blossom Fell | Nat King Cole | 2:32 |
| 15 | Autumn Leaves | Nat King Cole | 2:40 |
| 16 | Autumn Leaves (French version) | Nat King Cole | 2:36 |
| 17 | Autumn Leaves (Japanese version) | Nat King Cole | 2:44 |
| 18 | Stay as Sweet as You Are | Nat King Cole | 2:59 |
| 19 | Love Is a Many Splendored Thing | Nat King Cole | 2:42 |
| 20 | Mona Lisa | Nat King Cole | 3:16 |
| 21 | Quizas, Quizas, Quizas (Perhaps, Perhaps, Perhaps) | Nat King Cole | 2:45 |
| 22 | Non Dimenticar (Don't Forget) | Nat King Cole | 2:50 |
| 23 | Arrivederci Roma | Nat King Cole | 2:46 |
| 24 | Tu Sei Cosi Amabile (In Italian) | Nat King Cole | 2:49 |
| 25 | The Very Thought of You | Nat King Cole | 3:49 |
| 26 | On the Street Where You Live | Nat King Cole | 3:09 |
| 27 | Almost Like Being in Love | Nat King Cole | 1:55 |
| 28 | Somewhere Along the Way | Nat King Cole | 2:54 |
| 29 | Pretend | Nat King Cole | 2:44 |
| 30 | Tenderly | Nat King Cole | 2:59 |
| 31 | Darling, Je Vous Aime Beaucoup | Nat King Cole | 2:50 |
| 32 | Answer Me, My Love | Nat King Cole | 2:38 |
| 33 | Let There Be Love | Nat King Cole | 2:45 |
| 34 | Those Lazy, Hazy, Crazy Days of Summer | Nat King Cole | 2:25 |
| 35 | Wolverton Mountain | Nat King Cole | 3:04 |
| 36 | Ramblin' Rose | Nat King Cole | 2:50 |
| 37 | That Sunday, That Summer | Nat King Cole | 3:12 |
| 38 | When You're Smiling (The Whole World Smiles With You) | Nat King Cole | 2:44 |
| 39 | Fly Me to the Moon (In Other Words) | Nat King Cole & George Shearing | 3:32 |
| 40 | L-O-V-E | Nat King Cole | 2:34 |
| 41 | L-O-V-E (French version) | Nat King Cole | 2:32 |
| 42 | L-O-V-E (Italian version) | Nat King Cole | 2:34 |
| 43 | L-O-V-E (Japanese version) | Nat King Cole | 2:33 |
| 44 | Let's Face the Music and Dance | Nat King Cole | 2:26 |
| 45 | Just One of Those Things | Nat King Cole | 2:15 |
| 46 | Day In - Day Out | Nat King Cole | 2:26 |
| 47 | Thou Swell (live) | Nat King Cole | 2:05 |
| 48 | It's All in the Game | Nat King Cole | 3:07 |
| 49 | Love Letters | Nat King Cole | 2:45 |
| 50 | When I Fall in Love | Nat King Cole | 3:10 |
| 51 | Unforgettable | Nat King Cole & Natalie Cole | 3:31 |
| 52 | Stardust | Nat King Cole | 3:13 |