| 1 | Ring of Fire | Johnny Cash | 2:38 |
| 2 | I Walk the Line | Johnny Cash | 2:56 |
| 3 | Folsom Prison Blues (Live at Folsom State Prison, Folsom, CA - January 1968) | Johnny Cash | 2:41 |
| 4 | Highwayman | Johnny Cash , The Highwaymen , Willie Nelson , Waylon Jennings , Kris Kristofferson | 3:03 |
| 5 | (Ghost) Riders in the Sky | Johnny Cash | 3:46 |
| 6 | A Boy Named Sue (Live at San Quentin State Prison, San Quentin, CA - February 1969) | Johnny Cash | 3:58 |
| 7 | Jackson | Johnny Cash, June Carter | 2:45 |
| 8 | One Piece at a Time | Johnny Cash, The Tennessee Three | 4:01 |
| 9 | Man in Black | Johnny Cash | 2:52 |
| 10 | Sunday Morning Coming Down (Live at Ryman Auditorium, Nashville, TN - July 1970) | Johnny Cash | 4:06 |
| 11 | Cocaine Blues (Live at Folsom State Prison, Folsom, CA - January 1968) | Johnny Cash | 3:03 |
| 12 | Ragged Old Flag | Johnny Cash | 3:08 |
| 13 | Don't Take Your Guns to Town | Johnny Cash | 3:02 |
| 14 | American Remains | Johnny Cash , The Highwaymen , Willie Nelson , Waylon Jennings , Kris Kristofferson | 4:07 |
| 15 | The General Lee | Johnny Cash | 2:52 |
| 16 | Orange Blossom Special | Johnny Cash | 3:06 |
| 17 | There Ain't No Good Chain Gang | Johnny Cash | 3:15 |
| 18 | I Still Miss Someone | Johnny Cash | 2:33 |
| 19 | It Ain't Me, Babe | Johnny Cash | 3:02 |
| 20 | She Used to Love Me a Lot | Johnny Cash | 3:08 |
| 21 | A Thing Called Love | Johnny Cash | 2:32 |
| 22 | Five Feet High and Rising | Johnny Cash | 1:47 |
| 23 | Tennessee Flat-Top Box | Johnny Cash | 2:59 |
| 24 | Sunday Morning Coming Down (Live) | Johnny Cash | 4:09 |
| 25 | Hey Porter | Johnny Cash | 2:20 |
| 26 | The Ballad of Ira Hayes | Johnny Cash | 4:07 |
| 27 | San Quentin (Live at San Quentin State Prison, San Quentin, CA - February 1969 Version 1) | Johnny Cash | 4:06 |
| 28 | If I Were a Carpenter | Johnny Cash, June Carter Cash | 3:00 |
| 29 | 25 Minutes to Go (Live at Folsom State Prison, Folsom, CA 1st Show - January 1968) | Johnny Cash | 3:31 |
| 30 | Flesh and Blood | Johnny Cash | 2:36 |
| 31 | I Got Stripes | Johnny Cash | 2:03 |
| 32 | The One on the Right Is on the Left | Johnny Cash | 2:47 |
| 33 | Song of the Patriot | Johnny Cash | 3:28 |
| 34 | The Legend of John Henry's Hammer | Johnny Cash | 8:26 |
| 35 | Out Among the Stars | Johnny Cash | 3:00 |
| 36 | Understand Your Man | Johnny Cash | 2:43 |
| 37 | All Over Again | Johnny Cash | 2:12 |
| 38 | Dark as the Dungeon (Live at Folsom State Prison, Folsom, CA - January 1968) | Johnny Cash | 3:07 |
| 39 | I'm Movin' On | Johnny Cash | 3:07 |
| 40 | Wanted Man | Johnny Cash | 2:50 |
| 41 | Long-Legged Guitar Pickin' Man | Johnny Cash, June Carter | 2:35 |
| 42 | Busted | Johnny Cash | 2:16 |
| 43 | I Drove Her Out of My Mind | Johnny Cash | 2:58 |
| 44 | The Rebel-Johnny Yuma | Johnny Cash | 1:51 |
| 45 | The Long Black Veil (Live at Folsom State Prison, Folsom, CA 1st Show - January 1968) | Johnny Cash | 3:57 |
| 46 | The Wall | Johnny Cash | 2:10 |
| 47 | Me and Bobby McGee (Live at Channel DR-TV, Copenhagen, Denmark - September 1971) | Johnny Cash | 3:05 |
| 48 | Send a Picture of Mother (Live at Folsom State Prison, Folsom, CA - January 1968) | Johnny Cash | 2:10 |
| 49 | The City of New Orleans | Johnny Cash | 3:41 |
| 50 | Help Me Make It Through the Night | Johnny Cash, June Carter Cash | 2:57 |
| 51 | Baby Ride Easy | Johnny Cash | 2:41 |
| 52 | Jim, I Wore a Tie Today | Johnny Cash | 2:46 |
| 53 | All I Do Is Drive | Johnny Cash | 2:09 |
| 54 | Wabash Cannonball | Johnny Cash | 2:38 |
| 55 | If I Told You Who It Was | Johnny Cash | 3:03 |
| 56 | Oney | Johnny Cash | 3:06 |
| 57 | Highway Patrolman | Johnny Cash | 5:19 |
| 58 | Committed To Parkview | Johnny Cash, The Tennessee Three | 3:16 |
| 59 | Give My Love to Rose | Johnny Cash | 2:21 |
| 60 | Don't Think Twice, It's All Right | Johnny Cash | 2:56 |
| 61 | These Are My People | Johnny Cash | 2:38 |
| 62 | Swing Low, Sweet Chariot | Johnny Cash | 1:52 |
| 63 | It's All Over | Johnny Cash | 1:56 |